Catalytic performance of Ni/MgO catalyst in methane dry reforming

Methane dry reforming to synthesis gas over nickel catalysts supported on magnesium oxide has been studied. The support was prepared via co-precipitation method using ammonia solution (20 wt in water) as the precipitating agent. 10 wt of Ni metal was impregnated to form Ni/MgO catalyst. The prepared...

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Main Authors: Al-Swai, B.M., Osman, N.B., Abdullah, B.
Format: Article
Institution: Universiti Teknologi Petronas
Record Id / ISBN-0: utp-eprints.20006 /
Published: American Institute of Physics Inc. 2017
Online Access: https://www.scopus.com/inward/record.uri?eid=2-s2.0-85031315016&doi=10.1063%2f1.5005361&partnerID=40&md5=cc0981a1a56cdeecc90810be8f17e6b7
http://eprints.utp.edu.my/20006/
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spelling utp-eprints.200062018-04-22T14:32:21Z Catalytic performance of Ni/MgO catalyst in methane dry reforming Al-Swai, B.M. Osman, N.B. Abdullah, B. Methane dry reforming to synthesis gas over nickel catalysts supported on magnesium oxide has been studied. The support was prepared via co-precipitation method using ammonia solution (20 wt in water) as the precipitating agent. 10 wt of Ni metal was impregnated to form Ni/MgO catalyst. The prepared catalyst was characterized by different techniques, such as XRD, BET, SEM, and TGA analysis. The effect of reaction conditions on the conversions of CH4 and CO2, selectivity of H2 and CO, and carbon deposition were investigated in a tabular furnace reactor. The catalyst afforded as high as 93 CH4 conversion at 900 °C. The catalyst has also shown excellent stability during reaction at relatively higher space velocity (1.8×104 ml g-1 h-1) and 800 °C reaction temperature. TGA characterization of spent catalyst has shown lesser magnitude of carbon deposition on the surface of the catalyst at 900 °C. © 2017 Author(s). American Institute of Physics Inc. 2017 Article PeerReviewed https://www.scopus.com/inward/record.uri?eid=2-s2.0-85031315016&doi=10.1063%2f1.5005361&partnerID=40&md5=cc0981a1a56cdeecc90810be8f17e6b7 Al-Swai, B.M. and Osman, N.B. and Abdullah, B. (2017) Catalytic performance of Ni/MgO catalyst in methane dry reforming. AIP Conference Proceedings, 1891 . http://eprints.utp.edu.my/20006/
institution Universiti Teknologi Petronas
collection UTP Institutional Repository
description Methane dry reforming to synthesis gas over nickel catalysts supported on magnesium oxide has been studied. The support was prepared via co-precipitation method using ammonia solution (20 wt in water) as the precipitating agent. 10 wt of Ni metal was impregnated to form Ni/MgO catalyst. The prepared catalyst was characterized by different techniques, such as XRD, BET, SEM, and TGA analysis. The effect of reaction conditions on the conversions of CH4 and CO2, selectivity of H2 and CO, and carbon deposition were investigated in a tabular furnace reactor. The catalyst afforded as high as 93 CH4 conversion at 900 °C. The catalyst has also shown excellent stability during reaction at relatively higher space velocity (1.8×104 ml g-1 h-1) and 800 °C reaction temperature. TGA characterization of spent catalyst has shown lesser magnitude of carbon deposition on the surface of the catalyst at 900 °C. © 2017 Author(s).
format Article
author Al-Swai, B.M.
Osman, N.B.
Abdullah, B.
spellingShingle Al-Swai, B.M.
Osman, N.B.
Abdullah, B.
Catalytic performance of Ni/MgO catalyst in methane dry reforming
author_sort Al-Swai, B.M.
title Catalytic performance of Ni/MgO catalyst in methane dry reforming
title_short Catalytic performance of Ni/MgO catalyst in methane dry reforming
title_full Catalytic performance of Ni/MgO catalyst in methane dry reforming
title_fullStr Catalytic performance of Ni/MgO catalyst in methane dry reforming
title_full_unstemmed Catalytic performance of Ni/MgO catalyst in methane dry reforming
title_sort catalytic performance of ni/mgo catalyst in methane dry reforming
publisher American Institute of Physics Inc.
publishDate 2017
url https://www.scopus.com/inward/record.uri?eid=2-s2.0-85031315016&doi=10.1063%2f1.5005361&partnerID=40&md5=cc0981a1a56cdeecc90810be8f17e6b7
http://eprints.utp.edu.my/20006/
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score 11.62408