Preparation of Metal Oxide-based Oxygen Carriers Supported with CeO2 and γ-Al2O3 for Chemical Looping Combustion
The development of efficient oxygen carriers (OCs) in chemical looping combustion (CLC) exhibited tremendous achievement considering inherent CO2 capture. The selectivity of CO2 in the CLC process depends on the performance of employed OCs during multiple redox cycles. Different types of OCs were pr...
| Main Authors: | Qasim, M., Ayoub, M., Aqsha, A., Zulfiqar, M. |
|---|---|
| Format: | Article |
| Institution: | Universiti Teknologi Petronas |
| Record Id / ISBN-0: | utp-eprints.23751 / |
| Published: |
John Wiley and Sons Inc
2021
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| Online Access: |
https://www.scopus.com/inward/record.uri?eid=2-s2.0-85102268580&doi=10.1002%2fceat.202000438&partnerID=40&md5=e0216dcaa23a7d4a68275a179bc6e217 http://eprints.utp.edu.my/23751/ |
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utp-eprints.237512021-08-19T10:01:55Z Preparation of Metal Oxide-based Oxygen Carriers Supported with CeO2 and γ-Al2O3 for Chemical Looping Combustion Qasim, M. Ayoub, M. Aqsha, A. Zulfiqar, M. The development of efficient oxygen carriers (OCs) in chemical looping combustion (CLC) exhibited tremendous achievement considering inherent CO2 capture. The selectivity of CO2 in the CLC process depends on the performance of employed OCs during multiple redox cycles. Different types of OCs were prepared, including 5wtNi/5wtCe/γ-Al2O3, 5wtLa/5wtCe/γ-Al2O3, and 5wtPr/5wtCe/γ-Al2O3, using the wet impregnation method and characterized by scanning electron microscopy/energy-dispersive X-ray spectroscopy, temperature-programmed reduction, and thermogravimetric analysis (TGA). The redox reactivity of OCs was investigated through TGA and tubular furnace reactor. The as-prepared OCs revealed higher thermal stability along with excellent oxygen capacity. Pr/Ce/γ-Al2O3-based OCs showed moderate oxygen capacity, which may increase by the addition of active metals. © 2021 Wiley-VCH GmbH John Wiley and Sons Inc 2021 Article NonPeerReviewed https://www.scopus.com/inward/record.uri?eid=2-s2.0-85102268580&doi=10.1002%2fceat.202000438&partnerID=40&md5=e0216dcaa23a7d4a68275a179bc6e217 Qasim, M. and Ayoub, M. and Aqsha, A. and Zulfiqar, M. (2021) Preparation of Metal Oxide-based Oxygen Carriers Supported with CeO2 and γ-Al2O3 for Chemical Looping Combustion. Chemical Engineering and Technology, 44 (4). pp. 782-787. http://eprints.utp.edu.my/23751/ |
| institution |
Universiti Teknologi Petronas |
| collection |
UTP Institutional Repository |
| description |
The development of efficient oxygen carriers (OCs) in chemical looping combustion (CLC) exhibited tremendous achievement considering inherent CO2 capture. The selectivity of CO2 in the CLC process depends on the performance of employed OCs during multiple redox cycles. Different types of OCs were prepared, including 5wtNi/5wtCe/γ-Al2O3, 5wtLa/5wtCe/γ-Al2O3, and 5wtPr/5wtCe/γ-Al2O3, using the wet impregnation method and characterized by scanning electron microscopy/energy-dispersive X-ray spectroscopy, temperature-programmed reduction, and thermogravimetric analysis (TGA). The redox reactivity of OCs was investigated through TGA and tubular furnace reactor. The as-prepared OCs revealed higher thermal stability along with excellent oxygen capacity. Pr/Ce/γ-Al2O3-based OCs showed moderate oxygen capacity, which may increase by the addition of active metals. © 2021 Wiley-VCH GmbH |
| format |
Article |
| author |
Qasim, M. Ayoub, M. Aqsha, A. Zulfiqar, M. |
| spellingShingle |
Qasim, M. Ayoub, M. Aqsha, A. Zulfiqar, M. Preparation of Metal Oxide-based Oxygen Carriers Supported with CeO2 and γ-Al2O3 for Chemical Looping Combustion |
| author_sort |
Qasim, M. |
| title |
Preparation of Metal Oxide-based Oxygen Carriers Supported with CeO2 and γ-Al2O3 for Chemical Looping Combustion |
| title_short |
Preparation of Metal Oxide-based Oxygen Carriers Supported with CeO2 and γ-Al2O3 for Chemical Looping Combustion |
| title_full |
Preparation of Metal Oxide-based Oxygen Carriers Supported with CeO2 and γ-Al2O3 for Chemical Looping Combustion |
| title_fullStr |
Preparation of Metal Oxide-based Oxygen Carriers Supported with CeO2 and γ-Al2O3 for Chemical Looping Combustion |
| title_full_unstemmed |
Preparation of Metal Oxide-based Oxygen Carriers Supported with CeO2 and γ-Al2O3 for Chemical Looping Combustion |
| title_sort |
preparation of metal oxide-based oxygen carriers supported with ceo2 and î³-al2o3 for chemical looping combustion |
| publisher |
John Wiley and Sons Inc |
| publishDate |
2021 |
| url |
https://www.scopus.com/inward/record.uri?eid=2-s2.0-85102268580&doi=10.1002%2fceat.202000438&partnerID=40&md5=e0216dcaa23a7d4a68275a179bc6e217 http://eprints.utp.edu.my/23751/ |
| _version_ |
1741196726288515072 |
| score |
11.62408 |