Extraction of palm kernel shell derived pyrolysis oil by supercritical carbon dioxide: Evaluation and modeling of phenol solubility

The extraction and recovery of value-added chemical compounds, such as phenolic compounds present in bio-oil has been a vital subject of study recently. In this work, the extraction of bio-oil using supercritical carbon dioxide (sc-CO2) with particular interest in apparent solubility of phenol (a ma...

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Main Authors: Chan, Y.H., Yusup, S., Quitain, A.T., Chai, Y.H., Uemura, Y., Loh, S.K.
Format: Article
Institution: Universiti Teknologi Petronas
Record Id / ISBN-0: utp-eprints.21424 /
Published: Elsevier Ltd 2018
Online Access: https://www.scopus.com/inward/record.uri?eid=2-s2.0-85048734180&doi=10.1016%2fj.biombioe.2018.06.009&partnerID=40&md5=403c9e77cecbd3c51f63903f6ebf488f
http://eprints.utp.edu.my/21424/
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spelling utp-eprints.214242018-10-23T00:56:44Z Extraction of palm kernel shell derived pyrolysis oil by supercritical carbon dioxide: Evaluation and modeling of phenol solubility Chan, Y.H. Yusup, S. Quitain, A.T. Chai, Y.H. Uemura, Y. Loh, S.K. The extraction and recovery of value-added chemical compounds, such as phenolic compounds present in bio-oil has been a vital subject of study recently. In this work, the extraction of bio-oil using supercritical carbon dioxide (sc-CO2) with particular interest in apparent solubility of phenol (a major chemical compound in pyrolysis oil) was evaluated at various temperatures (50, 60 and 70 °C) and pressures (30, 35 and 40 MPa). Highest extraction yield of bio-oil was obtained at 70 °C and 40 MPa. The phenol content in the extracted bio-oils were also studied and reported. As a preliminary study, the apparent solubility data of phenol in sc-CO2 was successfully modeled using the values from the correlation of Chrastil, Adachi & Lu and Bartle models. The model parameters for these equations were determined and reported in this work. It was found that Chrastil, Adachi & Lu and Bartle models produced satisfactory correlations on the solubility of phenol in sc-CO2, with AARD values of 1.51, 6.52 and 1.85, respectively. © 2018 Elsevier Ltd Elsevier Ltd 2018 Article PeerReviewed https://www.scopus.com/inward/record.uri?eid=2-s2.0-85048734180&doi=10.1016%2fj.biombioe.2018.06.009&partnerID=40&md5=403c9e77cecbd3c51f63903f6ebf488f Chan, Y.H. and Yusup, S. and Quitain, A.T. and Chai, Y.H. and Uemura, Y. and Loh, S.K. (2018) Extraction of palm kernel shell derived pyrolysis oil by supercritical carbon dioxide: Evaluation and modeling of phenol solubility. Biomass and Bioenergy, 116 . pp. 106-112. http://eprints.utp.edu.my/21424/
institution Universiti Teknologi Petronas
collection UTP Institutional Repository
description The extraction and recovery of value-added chemical compounds, such as phenolic compounds present in bio-oil has been a vital subject of study recently. In this work, the extraction of bio-oil using supercritical carbon dioxide (sc-CO2) with particular interest in apparent solubility of phenol (a major chemical compound in pyrolysis oil) was evaluated at various temperatures (50, 60 and 70 °C) and pressures (30, 35 and 40 MPa). Highest extraction yield of bio-oil was obtained at 70 °C and 40 MPa. The phenol content in the extracted bio-oils were also studied and reported. As a preliminary study, the apparent solubility data of phenol in sc-CO2 was successfully modeled using the values from the correlation of Chrastil, Adachi & Lu and Bartle models. The model parameters for these equations were determined and reported in this work. It was found that Chrastil, Adachi & Lu and Bartle models produced satisfactory correlations on the solubility of phenol in sc-CO2, with AARD values of 1.51, 6.52 and 1.85, respectively. © 2018 Elsevier Ltd
format Article
author Chan, Y.H.
Yusup, S.
Quitain, A.T.
Chai, Y.H.
Uemura, Y.
Loh, S.K.
spellingShingle Chan, Y.H.
Yusup, S.
Quitain, A.T.
Chai, Y.H.
Uemura, Y.
Loh, S.K.
Extraction of palm kernel shell derived pyrolysis oil by supercritical carbon dioxide: Evaluation and modeling of phenol solubility
author_sort Chan, Y.H.
title Extraction of palm kernel shell derived pyrolysis oil by supercritical carbon dioxide: Evaluation and modeling of phenol solubility
title_short Extraction of palm kernel shell derived pyrolysis oil by supercritical carbon dioxide: Evaluation and modeling of phenol solubility
title_full Extraction of palm kernel shell derived pyrolysis oil by supercritical carbon dioxide: Evaluation and modeling of phenol solubility
title_fullStr Extraction of palm kernel shell derived pyrolysis oil by supercritical carbon dioxide: Evaluation and modeling of phenol solubility
title_full_unstemmed Extraction of palm kernel shell derived pyrolysis oil by supercritical carbon dioxide: Evaluation and modeling of phenol solubility
title_sort extraction of palm kernel shell derived pyrolysis oil by supercritical carbon dioxide: evaluation and modeling of phenol solubility
publisher Elsevier Ltd
publishDate 2018
url https://www.scopus.com/inward/record.uri?eid=2-s2.0-85048734180&doi=10.1016%2fj.biombioe.2018.06.009&partnerID=40&md5=403c9e77cecbd3c51f63903f6ebf488f
http://eprints.utp.edu.my/21424/
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